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Ring-Opening Metathesis Polymerization of the Dewar Isomer of 1,2-Azaborinine, a B–N Isostere of Benzene

https://doi.org/10.1021/acsmacrolett.3c00601

Lin, Huina ; Yang, Xinyu ; Liu, Shih-Yuan ; Jäkle, Frieder ( December 2023 , ACS Macro Letters)

The successful polymerization of the Dewar isomer of an azaborinine heterocycle is reported. Controlled ring-opening metathesis polymerization was accomplished with Grubbs and Hoveya−Grubbs second generation catalysts (G2, HG2), as well as a Z-selective Ru catalyst (HGM2001). The structure of the polymers containing 4-membered B−N heterocycles was verified by GPC and multinuclear and 2D NMR. Differences in stereochemistry of polymers derived from G2/HG2 versus the Z-selective catalyst HGM2001 were substantiated by 2D NOESY, FT-IR, and Raman analyses. The incorporation of B−N heterocycles into these polymer structures is promising as a route to functional polymers that contain polar side groups.
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Free, publicly-accessible full text available December 14, 2024
Stability Analysis of Substituted Cobaltocenium [Bis(cyclopentadienyl)cobalt(III)] Employing Chemistry-Informed Neural Networks

https://doi.org/10.1021/acs.jctc.1c01201

Li, Chunyan ; Wetthasinghe, Shehani T. ; Lin, Huina ; Zhu, Tianyu ; Tang, Chuanbing ; Rassolov, Vitaly ; Wang, Qi ; Garashchuk, Sophya ( May 2022 , Journal of Chemical Theory and Computation)

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Synthesis of cationic cobaltocenophane monomers: Isomerization and ring-opening metathesis polymerization

https://doi.org/10.1016/j.polymer.2022.124544

Cha, Yujin ; Hwang, JiHyeon ; Ramos, Luis ; Lin, Huina ; Zhu, Tianyu ; Tang, Chuanbing ( March 2022 , Polymer)

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Correlation between the Stability of Substituted Cobaltocenium and Molecular Descriptors

https://doi.org/10.1021/acs.jpca.1c10603

Wetthasinghe, Shehani T. ; Li, Chunyan ; Lin, Huina ; Zhu, Tianyu ; Tang, Chuanbing ; Rassolov, Vitaly ; Wang, Qi ; Garashchuk, Sophya ( January 2022 , The Journal of Physical Chemistry A)

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Mechanochemistry of Cationic Cobaltocenium Mechanophore

https://doi.org/10.1021/jacs.1c05233

Cha, Yujin ; Zhu, Tianyu ; Sha, Ye ; Lin, Huina ; Hwang, JiHyeon ; Seraydarian, Matthew ; Craig, Stephen L. ; Tang, Chuanbing ( August 2021 , Journal of the American Chemical Society)

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Tailored Triarylborane Polymers as Supported Catalysts and Luminescent Materials

https://doi.org/10.1021/acs.macromol.0c02258

Lin, Huina ; Patel, Shivani ; Jäkle, Frieder ( December 2020 , Macromolecules)
null (Ed.)
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Polysiloxane/Polystyrene Thermo-Responsive and Self-Healing Polymer Network via Lewis Acid-Lewis Base Pair Formation

https://doi.org/10.3390/molecules23020405

Vidal, Fernando ; Lin, Huina ; Morales, Cecilia ; Jäkle, Frieder ( February 2018 , Molecules)

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